1,412 research outputs found

    Critical current anisotropy in Nd-1111 single crystals and the infuence of neutron irradiation

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    We report on angle-resolved magnetization measurements on NdFeAsO0.65_{0.65}F0.35_{0.35} (Nd-1111) single crystals. The field dependence of the critical current density, JcJ_c, is non-monotonous in these crystals at all orientations and temperatures due to the fishtail effect, which strongly influences the angular dependence of JcJ_c. The currents decrease as the field is tilted from the crystallographic c-axis at low fields, but increase at high fields. A peak occurs in the angular dependence of JcJ_c at intermediate fields. The critical currents are significantly enhanced after irradiation with fast neutrons and the fishtail disappears. The different current anisotropies at low and high fields, however, persist. We discuss the data in the framework of the anisotropic scaling approach and propose a transition from dominant pinning by large defects of low density at low fields to pinning by small defects of high density at high fields in the pristine crystal. Strong pinning dominates at all fields after the irradiation, and the angular dependence of JcJ_c can be described by anisotropic scaling only after an appropriate extension to this pinning regime

    Pressure-induced lattice instabilities and superconductivity in YBa2Cu4O8 and optimally doped YBa2Cu3O7-{\delta}

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    Combined synchrotron angle-dispersive powder diffraction and micro-Raman spectroscopy are used to investigate the pressure-induced lattice instabilities that are accompanied by Tc_{\rm c} anomalies in YBa2_{\rm 2}Cu4_{\rm 4}O8_{\rm 8}, in comparison with the optimally doped YBa2_{\rm 2}Cu3_{\rm 3}O7−δ_{\rm 7-\delta} and the non-superconducting PrBa2_{\rm 2}Cu3_{\rm 3}O6.92_{\rm 6.92}. In the first two superconducting systems there is a clear anomaly in the evolution of the lattice parameters and an increase of lattice disorder with pressure, that starts at ≈3.7GPa\approx3.7 GPa as well as irreversibility that induces a hysteresis. On the contrary, in the Pr-compound the lattice parameters follow very well the expected equation of state (EOS) up to 7 GPa. In complete agreement with the structural data, the micro-Raman data of the superconducting compounds show that the energy and width of the Ag_{\rm g} phonons show anomalies at the same pressure range where the lattice parameters deviate from the EOS and the average Cu2-Opl_{pl} bond length exhibits a strong contraction and correlate with the non-linear pressure dependence of Tc_{\rm c}. This is not the case for the non superconducting Pr sample, clearly indicating a connection with the charge carriers. It appears that the cuprates close to optimal doping are at the edge of lattice instability.Comment: 6 pages, 7 figure
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